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COLLECTIVE SPIN EXCITATIONS OF ALKALI-METAL CLUSTERS

1993

The response function of alkali-metal clusters, modeled as jellium spheres, to dipole (L=1) and quadrupole (L=2) spin-dependent fields is obtained within the time-dependent local-spin-density approximation of density-functional theory. We predict the existence of low-energy spin modes of surface type, which are identified from the strength function. Their collectivity and evolution with size are discussed.

PhysicsCondensed matter physicsJelliumTeoria molecularFunction (mathematics)Alkali metalAtomic and Molecular Physics and OpticsDipolePhysical chemistryQuadrupoleQuasiparticleMolecular theorySPHERESCondensed Matter::Strongly Correlated ElectronsSpin (physics)Fisicoquímica
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